Scientific Highlights from Research Division
Research with Neutrons and Muons (NUM)
We have used neutron spectroscopy to investigate the spin dynamics of the quantum (S=1/2) antiferromagnetic Ising chains in RbCoCl3. The structure and magnetic interactions in this material conspire to produce two magnetic phase transitions at low temperatures, presenting an ideal opportunity for thermal control of the chain environment. The high-resolution spectra we measure ...
Phase boundary dynamics of bubble flow in a thick liquid metal layer under an applied magnetic field
We investigate argon bubble flow in liquid gallium within a container large enough to avoid wall effects. Flow with and without applied horizontal magnetic field is studied. We demonstrate the successful capture and quantification of the effects of applied magnetic field using dynamic neutron radiography and the previously developed and validated robust image processing pipeline, supported by the in silico reproduction of our experiment.
Simultaneous Nodal Superconductivity and Time-Reversal Symmetry Breaking in the Noncentrosymmetric Superconductor CaPtAs
By employing a series of experimental techniques, we provide clear evidence that CaPtAs represents a rare example of a noncentrosymmetric superconductor which simultaneously exhibits nodes in the superconducting gap and broken time-reversal symmetry (TRS) in its superconducting state (belowTc ≈ 1.5 K). Unlike in fully gapped superconductors, the magnetic penetration depth λ(T) does not saturate at low temperatures, but instead it shows a T2 dependence, characteristic of gap nodes.
In general, magnetism and superconductivity are antagonistic to each other. However, there are several families of superconductors in which superconductivity coexists with magnetism, and a few examples are known where the superconductivity itself induces spontaneous magnetism. The best known of these compounds are Sr2RuO4 and some non-centrosymmetric superconductors. Here, we report the finding of ...
The ancient purple pigment used to paint the terracotta warriors, BaCuSi2O6, is also a quantum magnetic material which consists of stacked Cu2+ bilayers hosting spin dimers. Magnetometry and NMR experiments have revealed puzzling critical phenomena at the quantum phase transition (QPT) caused by an applied magnetic field, which suggest that the universal behaviour of the system is not three- but only two-dimensional. By performing high-resolution neutron spectroscopy measurements .....
LaTiOxNy oxynitride thin films are employed to study the surface modifications at the solid- liquid interface that occur during photoelectrocatalytic water splitting. Neutron reflectometry and grazing incidence x-ray absorption spectroscopy were utilised to distinguish between the surface and bulk signals, with a surface sensitivity of 3 nm.
Elucidating the role of different degrees of freedom in a phase transition is crucial in the comprehension of complex materi- als. A phase transformation that attracts significant interest is the insulator-to-metal transition of Mott insulators, in which the electrons are thought to play the dominant role. Here, we use ultrafast laser spectroscopy and theoretical calculations ....
With experimental work demonstrating that the correlated ground state of the pyrochlore system Ce2Sn2O7 is a quantum liquid of magnetic octupoles, an international team led by PSI researcher Romain Sibille establishes a fundamentally new state of matter: higher-rank multipole ice.
We show that hybrid MnOx/C60 heterojunctions can be used to design a storage device for spin-polarized charge: a spin capacitor. Hybridization at the carbon-metal oxide interface leads to spin-polarized charge trapping after an applied voltage or photocurrent. Strong electronic structure changes, including a 1-eV energy shift and spin polarization in the C60 lowest unoccupied molecular orbital, are then revealed by x-ray absorption spectroscopy, in agreement with density functional theory simulations.
Detailed understanding of charge diffusion processes in a lithium-ion battery is crucial to enable its systematic improvement. Experimental investigation of diffusion at the interface between active particles and the electrolyte is challenging but warrants investigation as it can introduce resistances that, for example, limit the charge and discharge rates. Here, we show an approach to study diffusion at interfaces using muon spin spectroscopy.
Spin-based logic architectures provide nonvolatile data retention, near-zero leakage, and scalability, extending the technology roadmap beyond complementary metal–oxide–semiconductor logic. Architectures based on magnetic domain walls take advantage of the fast motion, high density, non-volatility and flexible design of domain walls to process and store information. Such schemes, however, rely on domain-wall manipulation and clocking using an external magnetic field, which limits their implementation in dense, large-scale chips.
Topological properties of materials are of fundamental as well as practical importance. Of particular interest are unconven- tional superconductors that break time-reversal symmetry, for which the superconducting state is protected topologically and vortices can host Majorana fermions with potential use in quantum computing. However, in striking contrast to the unconventional A phase of superfluid 3He where chiral symmetry was directly observed, .....
Forschende haben an der Quelle für ultrakalte Neutronen des PSI eine Eigenschaft des Neutrons so genau wie noch nie vermessen: sein elektrisches Dipolmoment. Denn bis heute wird nach einer Erklärung gesucht, weshalb es nach dem Urknall mehr Materie als Antimaterie gab.
Mit einer neu entwickelten Untersuchungsmethode konnten Forschende die magnetische Struktur im Inneren eines Materials mit Nanometer-Auflösung abbilden. Ihnen gelang ein kurzer «Film» aus sieben Bildern, der erstmalig in 3-D zeigt, wie sich winzige Wirbel der Magnetisierung tief im Inneren eines Materials verändern.
We report a comprehensive muon spin rotation (μSR) study of the prototypical magnetoelectric antiferromagnet Cr2O3. We find the positively charged muon (μ+) occupies several distinct interstitial sites and displays a rich dynamic behavior involving local hopping, thermally activated site transitions, and the formation of a charge-neutral complex composed of a muon and an electron polaron.
Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet
Magnetic topological phases of quantum matter are an emerging frontier in physics and material science. Along these lines, several kagome magnets have appeared as the most promising platforms. Here, we explore magnetic correlations in the kagome magnet Co3Sn2S2. Using muon spin-rotation, we present evidence for competing magnetic orders in the kagome lattice of this compound.
Possible room-temperature signatures of unconventional 4f-electron quantum criticality in YbMn6Ge6−xSnx
We investigate the Sn composition dependence of the Yb valence and local magnetization in YbMn6Ge6−xSnx (4.25 ≤x≤ 5.80) using x-ray absorption spectroscopy (XANES) and x-ray magnetic circular dichroism at the Yb L3 edge. In these materials, where Mn is ferromagnetically ordered, we observe a decrease of the Yb valence upon reducing the chemical pressure by Sn doping and a suppression of the Yb magnetic moment for strongly hybridized 4f states (ν ∼ 2.77).
Magnetism and anomalous transport in the Weyl semimetal PrAlGe: possible route to axial gauge fields
In magnetic Weyl semimetals, where magnetism breaks time-reversal symmetry, large magnetically sensitive anomalous transport responses are anticipated that could be useful for topological spintronics. The identification of new magnetic Weyl semimetals is therefore in high demand, particularly since in these systems Weyl node configurations may be easily modified using magnetic fields. Here we explore experimentally the magnetic semimetal PrAlGe, and unveil a direct correspondence between easy-axis Pr ferromagnetism and anomalous Hall and Nernst effects.
We report the discovery of topological magnetism in the candidate magnetic Weyl semimetal CeAlGe. Using neutron scattering we find this system to host several incommensurate, square-coordinated multi-k⃗ magnetic phases below TN. The topological properties of a phase stable at intermediate magnetic fields parallel to the c axis are suggested by observation of a topological Hall effect.
Forschende des Labors für Simulation und Modellierung des PSI lösen durch die Kombination von Theorie, Modellierung und Hochleistungsrechnen komplexeste Probleme. Mit leistungsfähigen Computern simulieren sie kleinste Moleküle oder Grossforschungsanlagen.