Scientific Highlights: Research Division "Research with Neutrons and Muons"

The basis for our understanding of quantum magnetism has been the study of elegantly simple model systems. However, even for the antiferromagnetic honeycomb lattice with isotropic spin interactions – one of the simplest model systems – a detailed understanding of quantum effects is still lacking. Here, using inelastic neutron scattering measurements of the honeycomb lattice material YbCl₃, we elucidate how quantum effects renormalize ...

Manipulating the spin state of thin layers of superconducting material is a promising route to generate dissipationless spin currents in spintronic devices. Approaches typically focus on using thin ferromagnetic elements to perturb the spin state of the superconducting condensate to create spin-triplet correlations. We have investigated simple structures that generate spin-triplet correlations without using ferromagnetic elements.

Kagome lattices are intriguing and rich platforms for studying the intertwining of topology, electron correlation, and magnetism. These materials have been subject to tremendous experimental and theoretical studies not only due to their exciting physical properties but also as systems that may solve critical technological problems. We will review recent experimental progress on superconductivity and magnetic fingerprints of charge order in several kagome-lattice systems from the local-magnetic probe point of view by utilizing muon-spin rotation under extreme conditions, i.e., hydrostatic pressure, ultra low temperature and high magnetic field.

Aliovalent doping is a way to optimize the electrical properties of semiconductors, but its impact on the phonon structure and propagation is seldom considered properly. Here we show that aliovalent doping can be much more effective in reducing the lattice thermal conductivity of thermoelectric semiconductors than the commonly employed isoelectronic alloying strategy. We demonstrate ...

The helical magnetic structures of cubic chiral systems are well explained by the competition among Heisen- berg exchange, Dzyaloshinskii-Moriya interaction, cubic anisotropy, and anisotropic exchange interaction (AEI). Recently, the role of the latter has been argued theoretically to be crucial for the low-temperature phase diagram of the cubic chiral magnet Cu₂OSeO₃, which features tilted conical and disordered skyrmion states for a specific orientation of the applied magnetic field (μ₀H⃗ ∥ [001]). In this study ...

The current challenge to realizing continuously tunable magnetism lies in our inability to systematically change properties, such as valence, spin, and orbital degrees of freedom, as well as crystallographic geometry. Here, we demonstrate that ferromagnetism can be externally turned on with the application of low-energy helium implantation and can be subsequently erased and returned to the pristine state via annealing.

In this paper we present a model system built out of artificially layered materials, allowing us to understand the interrelation of magnetic phases with the metallic-insulating phase at long length scales, and enabling new strategies for the design and control of materials in devices. The artificial model system consists of superlattices made of SmNiO₃ and NdNiO₃ layers, – two members of the fascinating rare earth nickelate family, having different metal-to-insulator and magnetic transition temperatures. By combining two complementary techniques ....

We report resonant elastic x-ray scattering of long-range magnetic order in EuPtSi₃, combining different scattering geometries with full linear polarization analysis to unambiguously identify magnetic scattering contributions. At low temperatures, EuPtSi₃ stabilizes type A antiferromagnetism featuring various long- wavelength modulations. For magnetic fields applied in the hard magnetic basal plane, well-defined regimes of cycloidal, conical, and fanlike superstructures may be distinguished that encompass a pocket of commensurate type A order without superstructure.

Muon spin rotation with low-energy muons (LE-μSR) is a powerful nuclear method where electrical and magnetic properties of surface-near regions and thin films can be studied on a length scale of ≈200 nm. This study shows the potential of utilizing low-energy muons for a depth-resolved characterization of oxide-semiconductor interfaces, i.e., for silicon (Si) and silicon carbide (4H-SiC). The performance of semiconductor devices relies heavily on the quality of the oxide-semiconductor interface; thus, investigation of defects present in this region is crucial to improve the technology.

Control of magnetization and electric polarization is attractive in relation to tailoring materials for data storage and devices such as sensors or antennae. In magnetoelectric materials, these degrees of freedom are closely coupled, allowing polarization to be controlled by a magnetic field, and magnetization by an electric field, but the magnitude of the effect remains a challenge in the case of single-phase magnetoelectrics for applications. 

The newly discovered kagome superconductors represent a promising platform for investigating the interplay between band topology, electronic order and lattice geometry. Despite extensive research efforts on this system, the nature of the superconducting ground state remains elusive. In particular, consensus on the electron pairing symmetry has not been achieved so far, in part owing to the lack of a momentum-resolved measurement of the superconducting gap structure. Here we report ...

It has long been hoped that spin liquid states might be observed in materials that realize the triangular-lattice Hubbard model. However, weak spin–orbit coupling and other small perturbations often induce conventional spin freezing or magnetic ordering. Sufficiently strong spin–orbit coupling, however, can renormalize the electronic wavefunction and induce anisotropic exchange interactions that promote magnetic frustration.

Neutron scattering experiments at three-axes spectrometers (TAS) investigate magnetic and lattice excitations by measuring intensity distributions to understand the origins of materials properties. The high demand and limited availability of beam time for TAS experiments however raise the natural question whether we can improve their efficiency and make better use of the experimenter’s time. 

Coacervation via liquid-liquid phase separation provides an excellent oppor- tunity to address the challenges of designing nanostructured biomaterials with multiple functionalities. Protein-polysaccharide coacervates, in particular, offer an appealing strategy to target biomaterial scaffolds, but these systems suffer from the low mechanical and chemical stabilities of protein-based condensates. Here we overcome these limitations by transforming native proteins into amyloid fibrils and demonstrate ...

Nanoscale thin films are widely implemented across a plethora of technological and scientific areas, and form the basis for many advancements that have driven human progress, owing to the high degree of functional tunability based on the chemical composition. Pulsed laser deposition is one of the multiple physical vapour deposition routes to fabricate thin films, employing laser energy to eject material from a target in the form of a plasma ...