Scientific Highlights

Magnetic topological phases of quantum matter are an emerging frontier in physics and materials science, of which kagome magnets appear as a highly promising platform. Here, we explore magnetic correlations in the recently identified topological kagome system TbMn₆Sn₆ using muon spin rotation, combined with local field analysis and neutron diffraction. Our studies identify an out-of-plane ferrimagnetic structure with slow magnetic fluctuations which exhibit a critical slowing down below T_^*C1 ≃ 120 K and finally freeze into static patches with ideal out-of-plane order below T_C1 ≃ 20 K....

The recently discovered kagome superconductor CsV₃Sb₅ (T_c ≃ 2.5 K) has been found to host charge order as well as a non-trivial band topology, encompassing multiple Dirac points and probable surface states. Such a complex and phenomenologically rich system is, therefore, an ideal playground for observing unusual electronic phases. Here, we report anisotropic superconducting properties of CsV₃Sb₅ by means of transverse-field muon spin rotation (μSR) experiments.

Many in-memory computing frameworks demand electronic devices with specific switching characteristics to achieve the desired level of computational complexity. Existing memristive devices cannot be reconfigured to meet the diverse volatile and non-volatile switching requirements, and hence rely on tailored material designs specific to the targeted application, limiting their universality. “Reconfigurable memristors” that combine both ionic diffusive and drift mechanisms could address these limitations, but they remain elusive. Here we present a reconfigurable halide perovskite nanocrystal memristor that achieves on-demand switching between diffusive/volatile and drift/non-volatile modes by controllable electrochemical reactions.

Static stripe order is detrimental to superconductivity. Yet, it has been proposed that transverse stripe fluctuations may enhance the inter-stripe Josephson coupling and thus promote superconductivity. Direct experimental studies of stripe dynamics, however, remain difficult. From a strong-coupling perspective, transverse stripe fluctuations are realized in the form of dynamic “kinks”—sideways shifting stripe sections. Here, we show how modest uniaxial pressure tuning reorganizes directional kink alignment.

Magnetic skyrmions are topologically stable swirling spin textures with particle-like char- acter, and have been intensively studied as a candidate of high-density information bit. While magnetic skyrmions were originally discovered in noncentrosymmetric systems with Dzyaloshinskii-Moriya interaction, recently a nanometric skyrmion lattice has also been reported for centrosymmetric rare-earth compounds, such as Gd₂PdSi₃ and GdRu₂Si₂. For the latter systems, a distinct skyrmion formation mechanism mediated by itinerant electrons has been proposed, and the search of a simpler model system allowing for a better understanding of their intricate magnetic phase diagram is highly demanded. Here, we report the discovery of square and rhombic lattices of nanometric skyrmions in a centrosymmetric binary compound EuAl₄, by performing small-angle neutron and resonant elastic X-ray scattering experiments.

Topological semimetals are three dimensional materials with symmetry-protected massless bulk excitations. As a special case, Weyl nodal-line semimetals are realized in materials having either no inversion or broken time-reversal symmetry and feature bulk nodal lines. The 111-family, including LaNiSi, LaPtSi and LaPtGe materials (all lacking inversion symmetry), belongs to this class. Here, by combining muon-spin rotation and relaxation with thermodynamic measurements, we find that these materials exhibit a fully- gapped superconducting ground state, while spontaneously breaking time-reversal symmetry at the superconducting transition.

Recent observations of novel spin-orbit coupled states have generated interest in 4d/5d transition metal systems. A prime example is the J_eff = 1/2 state in iridate materials and α-RuCl that drives Kitaev interactions. Here, by tuning the competition between spin-orbit interaction (λ_SOC) and trigonal crystal field (Δ_T), we restructure the spin-orbital wave functions into a previously unobserved μ=1/2 state that drives Ising interactions.

We present a new measurement of the bottom quark mass in the MS scheme at the renormalization scale of the Higgs boson mass from measurements of Higgs boson decay rates at the LHC: m_b (m_H) = 2.6 ^+0.36_-0.31 GeV. The measurement has a negligible theory uncertainty and excellent prospects to improve at the HL-LHC and a future Higgs factory.

Spin glasses, generally defined as disordered systems with randomized competing interactions, are a widely investigated complex system. Theoretical models describing spin glasses are broadly used in other complex systems, such as those describing brain function, error-correcting codes or stock-market dynamics. This wide interest in spin glasses provides strong motivation to generate an artificial spin glass within the framework of artificial spin ice systems. Here we present the experimental realization of an artificial spin glass consisting of dipolar coupled single-domain Ising-type nanomagnets arranged onto an interaction network that replicates the aspects of a Hopfield neural network.

Just as electrons flow through an electrical conductor, magnetic excitations can travel through certain materials. Such excitations, known in physics as "magnons" in analogy to the electron, could transport information much more easily than electrical conductors. An international research team has now made an important discovery on the way towards such components, which could be highly energy-efficient and considerably smaller.

Measurement of the absolute value of the applied pressure in high-pressure muon and neutron experiments is a complicated task. It often requires the presence of a calibration material inside the sample volume, and could also cause additional time to obtain the response of the calibrant. Here we describe the use of optical calibrants for precise determination of the pressure value inside the piston-cylinder clamp cells.

Excitonic insulators are usually considered to form via the condensation of a soft charge mode of bound electron-hole pairs. This, however, presumes that the soft exciton is of spin-singlet character. Early theoretical considerations have also predicted a very distinct scenario, in which the condensation of magnetic excitons results in an antiferromagnetic excitonic insulator state. Here we report resonant inelastic x-ray scattering (RIXS) measurements of Sr₃Ir₂O₇.

Muons are particles with a spin of 1⁄2 that can be implanted into a wide range of condensed matter materials to act as a local probe of the surrounding atomic environment. Measurement of the muon’s precession and relaxation provides an insight into how it interacts with its local environment. From this, unique information is obtained about the static and dynamic properties of the material of interest ...

Magnetoelectric phenomena are intimately linked to relativistic effects and also require the material to break spatial inversion symmetry and time-reversal invariance. Magnetoelectric coupling can substantially affect light–matter interaction and lead to non-reciprocal light propagation. Here, we confirm on a fully experimental basis, without invoking either symmetry-based or material-specific assumptions, that the optical magnetoelectric effect in materials with non-parallel magnetization (M) and electric polarization (P) generates a trilinear term in the refractive index...

We report a new measurement of the n=2 Lamb shift in Muonium. Our result of 1047.2(2.3)_stat(1.1)_syst  MHz comprises an order of magnitude improvement upon the previous best measurement. This value matches ...