LNS - Scientific Highlights

The interplay between oxygen and spin ordering for the low oxygen doped Nd₂NiO_4.10 has been investigated by single-crystal neutron diffraction. We find a coexistence of the magnetic order below T_N  with the 3D ordering of excess oxygen atoms, which has not been previously observed for the homologous nickelates. Moreover, the magnetic ordering modulation vectors are no longer independent and exactly follow the modulation vectors of the oxygen ordering.

Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T =0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin liquids have been predicted. Here, we experimentally study an effective S = 1/2 Heisenberg honeycomb lattice with competing nearest and next-nearest-neighbour interactions.

Magnetic skyrmion is a topologically protected particle-like object in magnetic materials, appearing as a nanometric swirling spin texture. The size and shape of skyrmion particles can be flexibly controlled by external stimuli, which suggests unique features of their crystallization and lattice transformation process. Here, we investigated the detailed mechanism of structural transition of skyrmion lattice (SkL) in a prototype chiral cubic magnet Cu₂OSeO₃, by combining resonant soft X-ray scattering (RSXS) experiment and micromagnetic simulation...

Quantum materials have properties that defy conventional theories of solids. Explaining these unusual properties is a frontier in physics, which promises both technological applications and fundamentally new states of matter. Yb₂Ti₂O₇ is a center of attention in this work. While it becomes ferromagnetic at very low temperature, its excitation spectrum resembles that of a quantum spin liquid. We show using neutron scattering ...

In the three-dimensional (3D) Heisenberg model, topological point defects known as spin hedgehogs behave as emergent magnetic monopoles, i.e., quantized sources and sinks of gauge fields that couple strongly to conduction electrons, and cause unconventional transport responses such as the gigantic Hall effect. We observe a dramatic change in the Hall effect upon the transformation of a spin hedgehog crystal in a chiral magnet MnGe through combined measurements of magnetotransport and small-angle neutron scattering (SANS).

Magnetic skyrmions are topological solitons with a nanoscale winding spin texture that hold promise for spintronics applications. Skyrmions have so far been observed in a variety of magnets that exhibit nearly parallel alignment for neighbouring spins, but theoretically skyrmions with anti-parallel neighbouring spins are also possible. Such antiferromagnetic skyrmions may allow more flexible control than conventional ferromagnetic skyrmions. Here, by combining neutron scattering measurements and Monte Carlo simulations, we show that a fractional antiferromagnetic skyrmion lattice is stabilized in MnSc₂S₄ through anisotropic couplings.

Noncollinear magnetic order arises for various reasons in several magnetic systems and exhibits interesting spin dynamics. Despite its ubiquitous presence, little is known of how magnons, otherwise stable quasiparticles, decay in these systems, particularly in metallic magnets. Using inelastic neutron scattering, we examine the magnetic excitation spectra in a metallic noncollinear antiferromagnet CrB₂, in which Cr atoms form a triangular lattice and display incommensurate magnetic order. Our data show intrinsic magnon damping ...