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Publications 2017

Publications 2017

Operando X-ray absorption spectroscopy: A powerful tool toward water splitting catalyst development E. Fabbri, D.F. Abbott, M. Nachtegaal, T.J. Schmidt
Current Opinion in Electrochemistry 5, 20-26 (2017).
DOI: 10.1016/j.coelec.2017.08.009OG-5423
 
Microstructure-property relationships in a gas diffusion layer (GDL) for Polymer Electrolyte Fuel Cells, Part II: pressure-induced water injection and liquid permeability L. Holzer, O. Pecho, J. Schumacher, Ph. Marmet, F.N. Büchi, A. Lamibrac, B. Münch
Electrochim. Acta 241, 414-432 (2017).
DOI: 10.1016/j.electacta.2017.04.141OG-5422
 
Microstructure-property relationships in a gas diffusion layer (GDL) for Polymer Electrolyte Fuel Cells, Part I: effect of compression and anisotropy of dry GDL L. Holzer, O. Pecho, J. Schumacher, Ph. Marmet, O. Stenzel, F.N. Büchi, A. Lamibrac, B. Münch
Electrochim. Acta 227, 419-434 (2017).
DOI: 10.1016/j.electacta.2017.01.030OG-5422
 
Experimental and pore-level numerical investigation of water evaporation in gas diffusion layers of polymer electrolyte fuel cells M.A. Safi, N.I. Prasianakis, J. Mantzaras, A. Lamibrac, F.N. Büchi
Int. J. Heat Mass Transfer 115 Part A, 238-249 (2017).
DOI: 10.1016/j.ijheatmasstransfer.2017.07.050OG-5422
 
Electrochemical hydrogen compression: Efficient pressurization concept derived from an energetic evaluation M. Suermann, T. Kiupel, T.J. Schmidt, F.N. Büchi
J. Electrochem. Soc. 164 (12), F1187-F1195 (2017).
DOI: 10.1149/2.1361712jesOG-5422
 
Influence of operating conditions and material properties on the mass transport losses of polymer electrolyte water electrolysis M. Suermann, K. Takanohashi, A. Lamibrac, T.J. Schmidt, F.N. Büchi
J. Electrochem. Soc. 164 (9), F973-F980 (2017).
DOI: 10.1149/2.13517109jesOG-5422
 
Fighting the noise: Towards the limits of subsecond X-ray tomographic microscopy of PEFC H. Xu, M. Bührer, F. Marone, T.J. Schmidt, F.N. Büchi, J. Eller
ECS Trans. 80 (8), 395-402 (2017).
DOI: 10.1149/08008.0395ecstOG-5422
 
Operando monitoring of early Ni-mediated surface reconstruction in layered lithiated Ni–Co–Mn oxides D. Streich, C. Erk, A. Guéguen, P. Müller, F.-F. Chesneau, E.J. Berg
J. Phys. Chem. C 121 (25), 13481-13486 (2017).
DOI: 10.1021/acs.jpcc.7b02303OG-5410 , OG-5412
 
Hydrocarbon proton exchange membranes: Degradation and stabilization L. Gubler, W. Koppenol
The Chemistry of Membranes Used in Fuel Cells: Degradation and Stabilization, First Edition. John Wiley & Sons, Inc., ISBN 9781119196051, 12/17, 107-138 (2017).
DOI: 10.1002/9781119196082.ch5OG-5421
 
Crystal structure evolution via operando neutron diffraction during long-term cycling of a customized 5 V full Li-ion cylindrical cell LiNi0.5Mn1.5O4vs. graphite L. Boulet-Roblin, D. Sheptyakov, P. Borel, C. Tessier, P. Novák, C. Villevieille
J. Mater. Chem. A 5, 25574-25582 (2017).
DOI: 10.1039/C7TA07917FOG-5410 , OG-5411
 
Nanostructuring noble metals as unsupported electrocatalysts for polymer electrolyte fuel cells B. Cai, S. Henning, J. Herranz, T.J. Schmidt, A. Eychmüller
Adv. Energy Mater. 7, 1700548 (2017).
DOI: 10.1002/aenm.201700548OG-5423
 
Membrane architecture with ion-conducting channels through swift heavy ion induced graft copolymerization V. Sproll, M. Handl, R. Hiesgen, K.A. Friedrich, T.J. Schmidt, L. Gubler
J. Mater. Chem. A 5, 24826-24835 (2017).
DOI: 10.1039/C7TA07323BOG-5421
 
Cycling behavior of silicon-containing graphite electrodes, Part B: Effect of the silicon source T. Schott, R. Robert, S.Pacheco Benito, P.A. Ulmann, P. Lanz, S. Zürcher, M.E. Spahr, P. Novák, S. Trabesinger
J. Phys. Chem. C 121, 25718-25728 (2017).
DOI: 10.1021/acs.jpcc.7b08457OG-5410 , OG-5413
 
Elucidation of reaction mechanisms of Ni2SnP in Li-ion and Na-ion systems C. Marino, N. Dupré, C. Villevieille
J. Power Sources 365, 339-347 (2017).
DOI: 10.1016/j.jpowsour.2017.08.096OG-5410 , OG-5411
 
Interface and safety properties of phosphorus-based negative electrodes in Li-ion batteries C. Marino, M. El Kazzi, E.J. Berg, M. He, C. Villevieille
Chem. Mater. 29 (17), 7151-7158 (2017).
DOI: 10.1021/acs.chemmater.7b01128OG-5410 , OG-5411 , OG-5412 , OG-5414
 
Direct observation of active material interactions in flowable electrodes using X-ray tomography K.B. Hatzell, J. Eller, S.L. Morelly, M.H. Tang, N.J. Alvarez, Y. Gogotsi
Faraday Discuss. 199, 511-524 (2017).
DOI: 10.1039/C6FD00243AOG-5422
 
Tackling capacity fading in vanadium flow batteries with amphoteric membranes F. Oldenburg, T.J. Schmidt, L. Gubler
J. Power Sources 368, 68-72 (2017).
DOI: 10.1016/j.jpowsour.2017.09.051OG-5421
 
Electrochemical impedance spectroscopy of a Li–S battery: Part 2. Influence of separator chemistry on the lithium electrode/electrolyte interface J. Conder, C. Villevieille, S. Trabesinger, P. Novák, L. Gubler, R. Bouchet
Electrochim. Acta 255, 379-390 (2017).
DOI: 10.1016/j.electacta.2017.09.148OG-5410 , OG-5411 , OG-5413 , OG-5421
 
Capacitive electronic metal-support interactions: Outer surface charging of supported catalyst particles T. Binninger, T.J. Schmidt, D. Kramer
Phys. Rev. B 96 (16), 165405 (2017).
DOI: 10.1103/PhysRevB.96.165405OG-5423
 
Cycling behavior of silicon-containing graphite electrodes, Part A: Effect of the lithiation protocol T. Schott, R. Robert, P.A. Ulmann, P. Lanz, S. Zürcher, M.E. Spahr, P. Novák, S. Trabesinger
J. Phys. Chem. C 121 (34), 18423-18429 (2017).
DOI: 10.1021/acs.jpcc.7b05919OG-5410 , OG-5413
 
Boosting Pt oxygen reduction reaction activity by tuning the tin oxide support E. Fabbri, A. Rabis, Y. Chino, M. Uchida, T.J. Schmidt
Electrochem. Commun. 83, 90-95 (2017).
DOI: 10.1016/j.elecom.2017.09.006OG-5423
 
A new concept of an air-electrode catalyst for Li2O2 decomposition using MnO2 nanosheets on rechargeable Li-O2 batteries M. Saito, S. Kosaka, T. Fujinami, Y. Tachikawa, H. Shiroishi, D. Streich, E.J. Berg, P. Novák, S. Seki
Electrochim. Acta 252, 192-199 (2017).
DOI: 10.1016/j.electacta.2017.08.183OG-5410 , OG-5412
 
Dynamic surface self-reconstruction is the key of highly active perovskite nano-electrocatalysts for water splitting E. Fabbri, M. Nachtegaal, T. Binninger, X. Cheng, B.-J. Kim, J. Durst, F. Bozza, T. Graule, R. Schäublin, L. Wiles, M. Pertoso, N. Danilovic, K.E. Ayers, T.J. Schmidt
Nat. Mater. 16 (9), 925-931 (2017).
DOI: 10.1038/nmat4938OG-5423
 
Colloidal synthesis and electrochemistry of surface coated nano-LiNi0.80Co0.15Al0.05O2 R. Asakura, P. Novák, R. Robert
J. Electrochem. Soc. 164 (12), A2617-A2624 (2017).
DOI: 10.1149/2.1431712jesOG-5410 , OG-5414
 
Unsupported Pt-Ni aerogels with enhanced high current performance and durability in fuel cell cathodes S. Henning, H. Ishikawa, L. Kühn, J. Herranz, E. Müller, A. Eychmüller, T.J. Schmidt
Angew. Chem. Int. Ed. 56, 10707-10710 (2017).
DOI: 10.1002/anie.201704253OG-5423
 
Durability of unsupported Pt-Ni aerogels in PEFC cathodes S. Henning, J. Herranz, H. Ishikawa, B.J. Kim, D. Abbott, L. Kühn, A. Eychmüller, T.J. Schmidt
J. Electrochem. Soc. 164 (12), F1136-F1141 (2017).
DOI: 10.1149/2.0131712jesOG-5423
 
Comparative operando study of degradation mechanisms in carbon-based electrochemical capacitors with Li2SO4 and LiNO3 electrolytes K. Fic, M. He, E.J. Berg, P. Novák, E. Frackowiak
Carbon 120, 281-293 (2017).
DOI: 10.1016/j.carbon.2017.05.061OG-5410 , OG-5412
 
Amphoteric ion-exchange membranes with significantly improved vanadium barrier properties for all-vanadium redox flow batteries O. Nibel, T. Rojek, T.J. Schmidt, L. Gubler
ChemSusChem 10 (13), 2767-2777 (2017).
DOI: 10.1002/cssc.201700610OG-5421
 
Numerical partitioning model for the Koutecký-Levich analysis of electrochemical flow cells with a combined channel/wall-jet geometry S.A. Tschupp, S.E. Temmel, N. Poyatos Salguero, J. Herranz, T.J. Schmidt
J. Electrochem. Soc. 164 (11), E3448-E3456 (2017).
DOI: 10.1149/2.0441711jesOG-5423
 
State-of-the-art nanofabrication in catalysis K. Waiz, S.A. Tschupp, J. Herranz, T.J. Schmidt, Y. Ekinci, J.A. van Bokhoven
Chimia 71 (4), 160-169 (2017).
DOI: 10.2533/chimia.2017.160OG-5423
 
Highly active and stable iridium pyrochlores for oxygen evolution reaction D. Lebedev, M. Povia, K. Waltar, P.M. Abdala, I.E. Castelli, E. Fabbri, M.V. Blanco, A. Fedorov, C. Coperet, N. Marzari, T.J. Schmidt
Chem. Mater. 29 (12), 5182-5191 (2017).
DOI: 10.1021/acs.chemmater.7b00766OG-5423
 
Effect of ball milling on the electrocatalytic activity of Ba0.5Sr0.5Co0.8Fe0.2O3 towards the oxygen evolution reaction X. Cheng, E. Fabbri, B-J. Kim, M. Nachtegaal, T.J. Schmidt
J. Mater. Chem. A 5, 13130-13137 (2017).
DOI: 10.1039/c7ta00794aOG-5423
 
Effect of acid washing on the oxygen reduction reaction activity of Pt-​Cu aerogel catalysts S. Henning, L. Kuhn, J. Herranz, M. Nachtegaal, R. Hubner, M. Werheid, A. Eychmuller, T.J. Schmidt
Electrochim. Acta 233, 210-217 (2017).
DOI: 10.1016/j.electacta.2017.03.019OG-5423
 
Improved electrochemical performances of Li-rich nickel cobalt manganese oxide by partial substitution of Li+ by Mg2+ S. Sallard, D. Sheptyakov, C. Villevieille
J. Power Sources 359, 27–36 (2017).
DOI: 10.1016/j.jpowsour.2017.05.028OG-5410 , OG-5411
 
Surface and morphological investigation of the electrode/electrolyte properties in an all-solid-state battery using a Li2S-P2S5 solid electrolyte X. Wu, M. El Kazzi, C. Villevieille
J. Electroceram. 38, 1-8 (2017).
DOI: 10.1007/s10832-017-0084-zOG-5410 , OG-5411 , OG-5414
 
Elucidation of the reaction mechanisms of isostructural FeSn2 and CoSn2 negative electrodes for Na-ion batteries L.O. Vogt, C. Villevieille
J. Mater. Chem. A 5, 3865-3874 (2017).
DOI: 10.1039/C6TA10535AOG-5410 , OG-5411
 
Performance of different carbon electrode materials: Insights into stability and degradation under real vanadium redox flow battery operating conditions O. Nibel, S.M. Taylor, A. Pătru, E. Fabbri, L. Gubler, T.J. Schmidt
J. Electrochem. Soc. 164 (7), A1608-A1615 (2017).
DOI: 10.1149/2.1081707jesOG-5421 , OG-5423
 
Direct observation of lithium polysulfides in lithium–sulfur batteries using operando X-ray diffraction J. Conder, R. Bouchet, S. Trabesinger, C. Marino, L. Gubler, C. Villevieille
Nature Energy 2, 17069 (2017).
DOI: 10.1038/nenergy.2017.69OG-5410 , OG-5411 , OG-5421
 
Polyvinylamine-containing adsorbent by radiation-induced grafting of N-Vinylformamide onto ultrahigh molecular weight polyethylene films and hydrolysis for CO2 capture T. Rojek, L. Gubler, M.M. Nasef, E. Abouzari-Lotf
Ind. Eng. Chem. Res. 56 (20), 5925-5934 (2017).
DOI: 10.1021/acs.iecr.7b00862OG-5421
 
Electrochemical impedance spectroscopy of a Li–S battery: Part 1. Influence of the electrode and electrolyte compositions on the impedance of symmetric cells J. Conder, C. Villevieille, S. Trabesinger, P. Novák, L. Gubler, R. Bouchet
Electrochim. Acta 244, 61-68 (2017).
DOI: 10.1016/j.electacta.2017.05.041OG-5410 , OG-5411 , OG-5413 , OG-5421
 
Ligand influence in Li-ion battery hybrid active materials: Ni methylenediphosphonate vs. Ni dimethylamino methylenediphosphonate S. Schmidt, S. Sallard, D. Sheptyakov, P. Novák, C. Villevieille
Chem. Commun. 53, 5420-5423 (2017).
DOI: 10.1039/C7CC01982COG-5410 , OG-5411
 
High pressure polymer electrolyte water electrolysis: Test bench development and electrochemical analysis M. Suermann, A. Pătru, T.J. Schmidt, F.N. Buechi
Int. J. Hydrogen Energy 42 (17), 12076-12086 (2017).
DOI: 10.1016/j.ijhydene.2017.01.224OG-5422 , OG-5423
 
Unraveling thermodynamics, stability, and oxygen evolution activity of strontium ruthenium perovskite oxide B.-J. Kim, D.F. Abbott, X. Cheng, E. Fabbri, M. Nachtegaal, F. Bozza, I.E. Castelli, D. Lebedev, R. Schäublin, C. Copéret, T. Graule, N. Marzari, T.J. Schmidt
ACS Catal. 7 (5), 3245-3256 (2017).
DOI: 10.1021/acscatal.6b03171OG-5423
 
Impact of cobalt content in Na0.67MnxFeyCozO2 (x + y + z = 1), a cathode material for sodium ion batteries C. Marino, E. Marelli, C. Villevieille
RSC Adv. 7 (23), 13851-13857 (2017).
DOI: 10.1039/C7RA00566KOG-5410 , OG-5411
 
Stabilization of Pt nanoparticles due to electrochemical transistor switching of oxide support conductivity T. Binninger, R. Mohamed, A. Patru, K. Waltar, E. Gericke, X. Tuaev, E. Fabbri, P. Levecque, A. Hoell, T.J. Schmidt
Chem. Mater. 29 (7), 2831-2843 (2017).
DOI: 10.1021/acs.chemmater.6b04851OG-5423
 
Unraveling the interaction mechanism between amidoxime groups and vanadium ions at various pH conditions O. Nibel, M. Bon, M.L. Agiorgousis, T. Laino, L. Gubler, T.J. Schmidt
J. Phys. Chem. C 121, 6436-6445 (2017).
DOI: 10.1021/acs.jpcc.6b12540OG-5421
 
Mask-assisted electron radiation grafting for localized through-volume modification of porous substrates: influence of electron energy on spatial resolution A. Forner-Cuenca, V. Manzi-Orezzoli, P.M. Kristiansen, L. Gubler, T.J. Schmidt
J. Rad. Phys. Chem. 135, 133-141 (2017).
DOI: 10.1016/j.radphyschem.2017.01.036OG-5420 , OG-5424
 
Silicone Nanofilament-Supported Mixed Nickel-Metal Oxides for AlkalineWater Electrolysis D.F. Abbott, M. Meier, G.R. Meseck, E. Fabbri, S. Seeger, T.J. Schmidt
J. Electrochem. Soc. 164, F203-F208 (2017).
DOI: 10.1149/2.0201704jesOG-5423
 
IrO2-​TiO2: a High-​Surface Area, Active and Stable Electrocatalyst for Oxygen Evolution Reaction E. Oakton, D. Lebedev, M. Povia, D.F. Abbott, E. Fabbri, A. Fedorov, M. Nachtegaal, C. Coperet, T.J. Schmidt
ACS Catal. 7, 2346-2352 (2017).
DOI: 10.1021/acscatal.6b03246OG-5423
 
Critical review—identifying critical Gaps for polymer electrolyte water electrolysis development U. Babic, M. Suermann, F.N. Büchi, L. Gubler, T.J. Schmidt
J. Electrochem. Soc. 164 (4), F387-F399 (2017).
DOI: 10.1149/2.1441704jesOG-5421 , OG-5422
 
Structural analysis and electrochemical properties of bimetallic palladium–platinum aerogels prepared by a two-step gelation process M. Oezaslan , A.-K. Herrmann, M. Werheid, A.I. Frenkel, M. Nachtegaal, C. Dosche, C. Laugier Bonnaud, H.C. Yilmaz, L. Kühn, E. Rhiel, N. Gaponik, A. Eychmüller, T.J. Schmidt
ChemCatChem 9, 798-808 (2017).
DOI: 10.1002/cctc.201600667OG-5423
 
Fe and Co methylene diphosphonates as conversion materials for Li-ion batteries S. Schmidt, S. Sallard, D. Sheptyakov, M. Nachtegaal, P. Novák, C. Villevieille
J. Power Sources 342, 879-885 (2017).
DOI: 10.1016/j.jpowsour.2016.12.090OG-5410 , OG-5411
 
CuSbS2 as a negative electrode material for sodium ion batteries C. Marino, T. Block, R. Pöttgen, C. Villevieille
J. Power Sources 342, 616-622 (2017).
DOI: 10.1016/j.jpowsour.2016.12.100OG-5410 , OG-5411
 
The counterintuitive impact of separator–electrolyte combinations on the cycle life of graphite–silicon composite electrodes T. Schott, J.L. Gómez-Cámer, Ch. Bünzli, S. Trabesinger, P. Novák
J. Power Sources 343, 142-147 (2017).
DOI: 10.1016/j.jpowsour.2017.01.055OG-5410 , OG-5413
 
Operando properties of gas diffusion layers: Saturation and liquid permeability J. Eller, J. Roth, F. Marone, M. Stampanoni, F.N. Büchi
J. Electrochem. Soc. 164 (2), F115-F126 (2017).
DOI: 10.1149/2.0881702jesOG-5422
 
Relationship between the properties and cycle Life of Si/C composites as performance-enhancing additives to graphite electrodes for Li-Ion batteries T. Schott, J.L. Gómez-Cámer, P. Novák, S. Trabesinger
J. Electrochem. Soc. 164 (2), A190-A203 (2017).
DOI: 10.1149/2.0701702jesOG-5410 , OG-5413
 
Influence of surface oxygen groups on V(II) oxidation reaction kinetics S.M. Taylor, A. Patru, E. Fabbri, T.J. Schmidt
Electrochem. Commun. 75, 13-16 (2017).
DOI: 10.1016/j.elecom.2016.12.003OG-5423
 

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