18 August 2017
PSI scientists have developed a new type of X-ray optics that allows for analyzing the emission in resonant inelastic x-ray scattering (RIXS) experiments. The new approach combines the energy dispersion with imaging capabilities. In a collaborative effort with research groups from Göttingen and Hamburg, two new classes of RIXS experiments, energy mapping and RIXS imaging, have been demonstrated.
9 August 2017
The advent of x-ray free electron lasers has extended the unique capabilities of resonant x-ray spectroscopy techniques to ultrafast time scales. Here, in collaboration between researchers from PSI, Sorbonne Universités, HASYLAB/DESY, Synchrotron SOLEIL, CNRS, and Uppsala University, we report on a novel experimental method that allows retrieving with a single x-ray pulse the time evolution of an ultrafast process, not only at a few discrete time delays, but continuously over an extended time window.
24 July 2017
Controlled motions of atoms using ultrashort electric field pulses allow to manipulated the properties of a material on ultrafast timescales. Here we show how metallic structures can be used to enhance a THz electric field pulse and track the induced atomic motions with ultrashort x-ray pulses emitted by a X-ray free electron laser.
24 May 2017
Metal nanostructures can be fabricated by irradiation of suitable metal organic precursor molecules with a focused X-ray beam. This novel techniques offer the advantage of energy-selective deposition by switching of the incident photon energy due to the non-linear photon absorption cross-section of the precursor molecules for resonant excitation.
22 May 2017
For decades, the mechanism of Mott phase in Ca2
has puzzled researchers. This material is a paradigmatic case of multi-band Mott physics including spin-orbit and Hund's coupling. Progress has been impeded by the lack of knowledge about the low-energy electronic structure. With our recent contribution, we provided-- using angle-resolved photoemission electron spectroscopy -- the band structure of the paramagnetic insulating phase of Ca2
21 March 2017
Turning the semimetal graphene into a technologically useful semiconductor is challenging. One way of opening a band gap is to cut graphene into nanometre-wide ribbons, but even atomic-level roughness at the ribbon edges can seriously degrade the mobility of charge carriers. Recent advances in on-surface chemistry have made it possible to obtain graphene nanoribbons with atomically precise edges through direct synthesis from molecular building blocks. Here, we report the synthesis, full structural and electronic characterization of 9-atom wide graphene nanoribbons with significantly improved electronic properties.
5 January 2017
Media Releases Energy and Environment Research Using Synchrotron Light Micro- and Nanotechnology
Eighty percent of all products of the chemical industry are manufactured with catalytic processes. Catalysis is also indispensable in energy conversion and treatment of exhaust gases. Industry is always testing new substances and arrangements that could lead to new and better catalytic processes. Researchers of the Paul Scherrer Institute PSI in Villigen and ETH Zurich have now developed a method for improving the precision of such experiments, which may speed up the search for optimal solutions.
9 November 2016
Single holmium atoms adsorbed on few monolayers of magnesium oxide are extraordinarily stable magnets. They retain a significant fraction of their magnetization when the external magnetic field is switched off. This has been shown recently in a study combining x-ray magnetic circular dichroism performed at the Swiss Light Source (SLS) and at the European Synchrotron Radiation Facility (ESRF) as well as scanning tunneling microscopy. The results open perspectives of storing and processing information at ultrahigh density.
11 October 2016
Media Releases Matter and Material Materials Research Research Using Synchrotron Light
The material neodymium nickel oxide is either a metal or an insulator, depending on its temperature. The possibility to control this transition electrically makes the material a potential candidate for transistors in modern electronic devices. By means of a sophisticated development of X-ray scattering, researchers at the Paul Scherrer Institute PSI have now been able to track down the cause of this transition: electrons around the oxygen atoms are rearranging.
20 October 2016
The first example of an insulating phase which is close to the superconducting phase in an iron-pnictide system has been recently observed in heavy Cu-doped NaFe1-x
CuxAs (x > 0.3). A combined study by angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations revealed that on-site Coulomb repulsion and enhanced Hund’s rule coupling are responsible for the insulating behavior. The results show that the insulating phase in NaFe0.5
As resembles the situation in the parent compounds of the high-Tc
19 July 2016
The use of spin-wave signals in future information processing devices can substantially reduce power consumption over present charge current based technologies. As part of an international research venture, scientists at PSI now introduced a concept to generate spin waves with nanoscale wavelengths exploiting the driven dynamics of magnetic vortex cores in magnetic heterostructures.
19 July 2016
Researchers from PSI and EPFL have demonstrated that the magnetization hysteresis and remanence of TbPc2
single-molecule magnets drastically depends on the substrate on which they are deposited. If a few atomic layers thick magnesium oxide film grown on a silver substrate is used, a record wide hysteresis and record large remanence can be obtained. Single-molecule magnets are attractive for molecular spintronics applications such as information processing or storage.
14 July 2016
Researchers have overcome a number of challenges in order to employ an advanced probe in the study of an unusual material, barium bismuth oxide (BaBiO3) – an insulating parent compound of a family of high-temperature superconductors known since the late 80s. In order to finally realize the experiments, the researchers grew and studied thin films of the material completely in situ under ultrahigh vacuum conditions. The results show that superconductivity in bismuth oxides emerges out of a novel insulating phase, where hole pairs located on combinations of the oxygen orbitals are coupled with distortions of the crystal lattice.
23 June 2016
Resonant magnetic scattering performed at the x-ray free electron laser facility LCLS (USA) has been used to investigate the magnetization dynamics of elemental Holmium. It is found that the demagnetization of conduction electrons and localized 4f magnetic moments have the same temporal evolution showing a strong coupling between the different magnetic moments.
11 April 2016
The Angle Resolved Photoemission Spectroscopy (ARPES) measurements performed on 2DEL at STO surface revealed that, at low carrier density, electrons are always accompanied by a quantized dynamic lattice deformation. Together with the electron, these phonon-cloud formed a new composite quasiparticle called Fröhlich polaron.
27. January 2016
Media Releases Matter and Material Research Using Synchrotron Light
Computers and other electronic devices account for a substantial portion of worldwide energy use. With today’s technologies, it is not possible to reduce this energy consumption significantly any further; chips in the energy-saving electronics of the future will hence have to be made from novel materials. Researchers at the Paul Scherrer Institute PSI have now found important clues in the search for such materials.