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Laboratory for Waste Management (LES)

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Publications 2002

BERNER U.
Project opalinus clay: radionuclide concentration limits in the near-field of a repository for spent fuel and vitrified high-level waste
PSI Bericht Nr. 02-22, Nagra NTB 02-10


BERNER U.
Project opalinus clay: radionuclide concentration limits in the cementitious near-field of an ILW repository
PSI Bericht Nr. 02-26, Nagra NTB 02-22


BONHOURE I., SCHEIDEGGER A., WIELAND E., DÄHN R.
Iodine species uptake by cement and CSH studied by I K-edge X-ray absorption spectroscopy
Radiochimica Acta 90, 647-651 (2002)


BRADBURY M.H., BAEYENS B.
Porewater chemistry in compacted re-saturated MX-80 bentonite: Physico-chemical characterisation and geochemical modelling
PSI Bericht Nr. 02-10, Nagra NTB 01-08


BRADBURY M.H., BAEYENS B.
Sorption of Eu on Na- and Ca-montmorillonites: Experimental investigations and modelling with cation exchange and surface complexation
Geochimica et Cosmochimica Acta 66, 2325-2334 (2002)

BRESSLER CH., SAES M., CHERGUI M., GROLIMUND D., ABELA R.
Towards structural dynamics research with ultrashort pulse lasers and synchrotron radiation
in: Femtochemistry and Temtobiology, A. Douhal and J. Santamaria, eds., World Scientific, Singapore, 449-458 (2002)

BRESSLER CH. SAES M., CHERGUI M. GROLIMUND D.,ABELA R. PATTISON PH.
Towards structural dynamics in condensed chemical systems exploiting ultrafast time-resolved X-Ray absorption spectroscopy
J. Chem. Phys. 116, 2955-2966 (2002)

CURTI E., DEGUELDRE C.
Solubility and hydrolysis of Zr oxides: a review and supplemental data
Radiochimica Acta 90, 801-804 (2002)

DÄHN R., SCHEIDEGGER A.M., MANCEAU A., CURTI E., BAEYENS B., BRADBURY M.H. AND CHATEIGNER D.
Th uptake on montmorillonite: A powder and polarized extended X-ray absorption fine structure (EXAFS) study
Journal of Colloid and Interface Science 249, 8-21 (2002)


DÄHN R., SCHEIDEGGER A.M., MANCEAU A. , SCHLEGEL M.L., BAEYENS B., BRADBURY M.H. MORALES M.
Neoformation of Ni phyllosilicate upon Ni uptake on montmorillonite: A kinetics study by powder and polarized extended X-ray absorption fine structure spectroscopy
Geochimica et Cosmochimica Acta 66, 2335-2347 (2002)


FLURY M., GIMMI TH.
Solute diffusion. In: Methods of soil analysis, Part 4-Physical methods
ed. by J.H. Dane and G.C. Topp, p. 1323-1348 (2002)

K. GERAEDTS K., BRUGGEMAN C., MAES A., VAN LOON L.R., ROSSBERG A., REICH T.
Evidence for the existence of Tc(IV)-humic substances species by X-ray absorption near - edge spectroscopy
Radiochimica Acta 90, 879-884 (2002)

HADERMANN J., HOSEMANN J.P., DE REYFF CH.
Mit Sicherheit entsorgt
Das PSI schafft Grundlagen zur Beurteilung von Standorten und Lagersystemen
ENET-NEWS-Dezember 2002, pp. 36-37

HENNIG C., REICH T., DÄHN R., SCHEIDEGGER A.M.
Structure of uranium sorption complexes at montmorillonite edge sites
Radiochimica Acta 90, 653-657 (2002)

HLAWATSCH S., GARBE-SCHÖNBERG C.D., LECHTENBERG F., MANCEAU A., TAMURA N., KULIK D.A., KERSTEN M.
Trace metal fluxes to ferromanganes nodules from the Western Baltic Sea as a record for long-term environmental changes
Chemical Geology 182, 697-709 (2002)

HUMMEL W., BERNER U., CURTI E., PEARSON F.J., THOENEN T.
Nagra/PSI Chemical Thermodynamic Data Base 01/01
Radiochimica Acta 90, 805-813 (2002)

HUMMEL W., BERNER U., CURTI E., PEARSON F.J., THOENEN T.
Nagra/PSI Chemical Thermodynamic Data Base 01/01
Nagra Technical Report NTB 02-16, Nagra, Wettingen, Switzerland, and Universal Publishers/uPublish.com, Parkland, Florida, USA, ISBN 158 112 620 4. (2002a)

JAKOB A.
Diffusion of tritiated water (HTO) and 22Na+-Ions through non-degraded hardened cement pastes-II. modelling results
PSI Bericht Nr. 02-21, Nagra NTB 02-15


KARPOV I.K., CHUDNENKO K.V., KULIK D.A., BYCHINSKII V.A.
The convex programming minimization of five thermodynamic potentials other than Gibbs energy in Geochemical Modeling
American Journal of Science 302, 281-311 (2002)

KULIK D.A., KERSTEN M.
Aqueous solubility diagrams for cementitious waste stabilization systems. 4. A carbonation model for Zn-doped calcium silicate hydrate by Gibbs Energy Minimization
Environmental Science & Technology 36, 2926-2931 (2002)

KULIK D.A.
Sorption modelling by Gibbs energy minimisation: Towards a uniform thermodynamic database for surface complexes of radionuclides
Radiochimica Acta 90, 815-832 (2002)

KULIK D.A.
Gibbs energy minimization approach to modeling sorption equilibria at the mineral-water interface: Thermodynamic relations for multi-site-surface complexation
American Journal of Science 302, 227-279 (2002)


KUREPIN V.A., KULIK D.A., HILTPOLD A., NICOLET M.
Thermodynamic modelling of Fe-Cr-Ni spinel formation at the light-water reactor conditions
PSI Bericht Nr. 02-04

MAZUREK M., JAKOB A.
Evidence for matrix diffusion in the TRUE-1 block at Äspö based on fracture characterisation and modelling of tracer tests
in: Radionuclide Retention in Geologic Media, Workshop Proceedings, Oskarshamn, Sweden, 7-9 May 2001, Nuclear Energy Agency, Paris, France, OECD 2002, 137-154 (2002)


PFINGSTEN, W.
Experimental and modeling indications for self-sealing of a cementitious L&ILW repository by calcite precipitation
Nuclear Technology 140(1), 63-82 (2002)


PFINGSTEN W., KISLITSIN S.
*Radionuclide migration from underground nuclear tests performed at the Lira facility, Kazakhstan - estimations by source term and transport modelling. ModelCARE 2002 : Calibration and reliability in groundwater modelling, (K. Kovar and Z. Hrkal, eds.), Prague, Czech Republic, June 16-20, 2002. Univerzita Karlova V Praze Nakladatelstvi Karolinum, Acta Universitatis Carolinae-Geologica 46(2/3), 461-466 (2002)

SCHUESSLER W., METZ V., LÜTZENKIRCHEN J., KIENZLER B., PFINGSTEN W.
Modelling of coupled transport reaction processes - summary and conclusions of the TRePro 2002 Workshop held at Karlsruhe
atw - Internationale Zeitschrift für Kernenergie 47(8/9), 668-669 (2002)

THORENZ C., KOSAKOWSKI G., KOLDITZ O., BERKOWITZ B.
An experimental and numerical investigation of saltwater movement in coupled saturated-partially saturated systems
Water Resources Research 38, No. 6, doi: 10.1029/2001WR000364 (2002)


TITS J., WIELAND E., BRADBURY M.H., ECKERT P., SCHAIBLE A.
The uptake of Eu(III) and Th(IV) by calcite under hyperalkaline conditions
PSI-Bericht Nr. 02-03, Nagra NTB 02-08


VULAVA V.M., KRETZSCHMAR R., BARMETTLER K., VOEGELIN A., GROLIMUND D., BORKOVEC M.
Cation Competition in a Natural Subsurface Material: Prediction of Transport Behavior
Water Resources Research 38, 7-1-7-7 (2002)

WIELAND E., TITS J., DOBLER J.P., SPIELER P.
The effect of a-isosaccharinic acid on the stability of and Th(IV) uptake by hardened cement paste.
Radiochimica Acta 90, 683-688 (2002)

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