3D magnetic nanostructures are of great interest due to the possibility to design novel properties and the benefits for both technological applications such as high-density data storage, as well as more fundamental studies.
One of the main challenges facing the realization of these three-dimensional systems is their fabrication, which includes the deposition of magnetic materials on 3D surfaces. In this work, the electroless deposition of Ni–Fe
on a 3D-printed, non-conductive microstructure is presented.
Understanding the relationship between entangled degrees of freedom (DOF) is a central problem in correlated materials and the possibility to influence their balance is promising toward realizing novel functionalities. In Sr2IrO4, the interaction between spin–orbit coupling and electron correlations induces an exotic ground state with magnetotransport properties promising for antiferromagnetic spintronics applications.
The driving force in materials to spontaneously form states with magnetic or electric order is of fundamental importance for basic research and device technology. The macroscopic properties and functionalities of these ferroics depend on the size, distribution and morphology of domains; that is, of regions across which such uniform order is maintained. Typically, extrinsic factors such as strain profiles, grain size or annealing procedures control the size and shape of the domains, whereas intrinsic parameters are often difficult to extract due to the complexity of a processed material. Here, we achieve this separation ...
At an interface between a topological insulator (TI) and a conventional superconductor (SC), superconductivity has been predicted to change dramatically and exhibit novel correlations. In particular, the induced superconductivity by an s-wave SC in a TI can develop an order parameter with a p-wave component. Here we present experimental evidence for an unexpected proximity-induced novel super- conducting state in a thin layer of the prototypical TI, Bi2Se3 proximity coupled to Nb.
Z3-vestigial nematic order due to superconducting fluctuations in the doped topological insulators NbxBi2Se3 and CuxBi2Se3
A state of matter with a multi-component order parameter can give rise to vestigial order. In the vestigial phase, the primary order is only partially melted, leaving a remaining symmetry breaking behind, an effect driven by strong classical or quantum fluctuations. Vestigial states due to primary spin and charge-density-wave order have been discussed in iron-based and cuprate materials. Here we present the observation of a partially melted superconductivity in which pairing fluctuations condense at a separate phase transition and form a nematic state with broken Z3, i.e., three-state Potts-model symmetry.
Simultaneous Nodal Superconductivity and Time-Reversal Symmetry Breaking in the Noncentrosymmetric Superconductor CaPtAs
By employing a series of experimental techniques, we provide clear evidence that CaPtAs represents a rare example of a noncentrosymmetric superconductor which simultaneously exhibits nodes in the superconducting gap and broken time-reversal symmetry (TRS) in its superconducting state (belowTc ≈ 1.5 K). Unlike in fully gapped superconductors, the magnetic penetration depth λ(T) does not saturate at low temperatures, but instead it shows a T2 dependence, characteristic of gap nodes.
LaTiOxNy oxynitride thin films are employed to study the surface modifications at the solid- liquid interface that occur during photoelectrocatalytic water splitting. Neutron reflectometry and grazing incidence x-ray absorption spectroscopy were utilised to distinguish between the surface and bulk signals, with a surface sensitivity of 3 nm.
Elucidating the role of different degrees of freedom in a phase transition is crucial in the comprehension of complex materi- als. A phase transformation that attracts significant interest is the insulator-to-metal transition of Mott insulators, in which the electrons are thought to play the dominant role. Here, we use ultrafast laser spectroscopy and theoretical calculations ....
Detailed understanding of charge diffusion processes in a lithium-ion battery is crucial to enable its systematic improvement. Experimental investigation of diffusion at the interface between active particles and the electrolyte is challenging but warrants investigation as it can introduce resistances that, for example, limit the charge and discharge rates. Here, we show an approach to study diffusion at interfaces using muon spin spectroscopy.