Scientific Highlights

High-pressure studies reveal a stark contrast between the superconducting properties of double-layer Ruddlesden-Popper (RP) nickelates La₂⁢PrNi₂⁢O₇ and La₃⁢Ni₂⁢O₇. While La₂⁢PrNi₂⁢O₇ exhibits bulk superconductivity, La₃⁢Ni₂⁢O₇ displays filamentary behavior, suggesting that superconductivity is confined to phase interfaces rather than the bulk. Since magnetism emerges ...

Exchange interactions are mediated via orbital overlaps across chemical bonds. Thus, modifying the bond angles by physical pressure or strain can tune the relative strength of competing interactions. Here we present a remarkable case of such tuning between the Heisenberg (J) and Kitaev (K) exchange, which respectively establish magnetically ordered and spin liquid phases on a honeycomb lattice. We observe ...

The pursuit of a unifying theory for non-BCS superconductivity has faced significant challenges. One approach to overcome such challenges is to perform systematic investigations into superconductors containing d-electron metals in order to elucidate their underlying mechanisms. Recently, the Sc₆MTe₂ (M = d-electron metal) family has emerged as a unique series of isostructural compounds exhibiting superconductivity across a range of 3d, 4d, and 5d electron systems. 

In this study, muon spin rotation, neutron diffraction, and magnetization techniques are employed to probe ...

The interplay between topology and superconductivity generated great interest in condensed matter physics. Here, we unveil an unconventional two-dimensional superconducting state in the Dirac nodal line semimetal ZrAs₂ which is exclusively con ned to the top and bottom surfaces within the crystal’s ab plane. 

As a remarkable consequence ...

Crystalline solids can become band insulators due to fully lled bands, or Mott insulators due to strong electronic correlations. While Mott insulators can theoretically occur in systems with an even number of electrons per unit cell, distinguishing them from band insulators experimentally has remained a longstanding challenge. 

In this work, we present ...

Two-dimensional (2D) kagome lattice metals are interesting because their corner sharing triangle structure enables a wide array of electronic and magnetic phenomena. Recently, post-growth annealing is shown to both suppress charge density wave (CDW) order and establish long-range CDW with the ability to cycle between states repeatedly in the kagome antiferromagnet FeGe. 

Here we perform ...

The anomalous Hall effect (AHE) has emerged as a key indicator of time-reversal symmetry breaking (TRSB) and topological features in electronic band structures. Absent of a magnetic field, the AHE requires spontaneous TRSB but has proven hard to probe due to averaging over domains. The anomalous component of the Hall effect is thus frequently derived from extrapolating the magnetic field dependence of the Hall response. We show ....

The observation of superconductivity in La₃Ni₂O_7–δ under pressure, following the suppression of a high-temperature density wave state, has attracted considerable attention. The nature of this density wave order was not clearly identified. Here we probe the magnetic response of the zero-pressure phase of La₃Ni₂O_7–δ as hydrostatic pressure is applied, and find that the apparent single density wave transition at zero applied pressure splits into two. The comparison of our muon-spin rotation ...

Skyrmions are particlelike vortices of magnetization with nontrivial topology, which are usually stabilized by Dzyaloshinskii-Moriya interactions (DMI) in noncentrosymmetric bulk materials. Exceptions are centrosymmetric Gd- and Eu-based skyrmion-lattice (SL) hosts with zero DMI, where both the SL stabilization mechanisms and magnetic ground states remain controversial. We address these here by investigating both the static and dynamical spin properties  ...

Antiferromagnets with exotic spin textures promise low-power spintronic devices with extremely high operating frequencies and resistance to external perturbations. In particular, the combination of highly tunable correlated electron physics, as in complex oxides, with metallicity and antiferromagnetism is desirable but exceedingly rare. LaNiO₃, the lone example of a perovskite nickelate which is metallic across all temperatures, has long been a promising candidate, but the antiferromagnetic metallic state has remained elusive. We demonstrate the emergence  ...

We experimentally study the evolution of the magnetic moment 𝑚 and exchange interaction 𝐽 as a function of hydrostatic pressure in the zero-field helimagnetic phase of the strongly correlated electron system MnSi. The suppression of magnetic order at ≈1.5  GPa is shown to arise from the 𝐽 collapse and not from a quantum fluctuations induced reduction of 𝑚. Our work provides benchmarks ...

Superconductivity and magnetism are often antagonistic in quantum matter, although their intertwining has long been considered in frustrated-lattice systems. Here we utilize scanning tunnelling microscopy and muon spin resonance to demonstrate time-reversal symmetry-breaking superconductivity in kagome metal Cs(V, Ta)₃Sb₅, where the Cooper pairing exhibits magnetism and is modulated by it. In the magnetic channel, we observe spontaneous internal magnetism ...

Superconductivity involving finite-momentum pairing can lead to spatial-gap and pair-density modulations, as well as Bogoliubov Fermi states within the superconducting gap. However, the experimental realization of their intertwined relations has been challenging. Here we detect chiral kagome superconductivity modulations with residual Fermi arcs in KV₃Sb₅ and CsV₃Sb₅ using normal and Josephson scanning tunnelling microscopy down to 30 millikelvin with a resolved electronic energy difference at the microelectronvolt level. We observe a U-shaped ...

Two-dimensional magnetic materials can exhibit new magnetic properties due to the enhanced spin fluctuations that arise in reduced dimension. However, the suppression of the long-range magnetic order in two dimensions due to long-wavelength spin fluctuations, as suggested by the Mermin-Wagner theorem, has been questioned for finite-size laboratory samples. Here we study ...

The interface of two materials can harbor unexpected emergent phenomena. One example is interface-induced superconductivity. In this work, we employ molecular beam epitaxy to grow a series of heterostructures formed by stacking together two nonsuperconducting antiferromagnetic materials, an intrinsic antiferromagnetic topological insulator MnBi₂Te₄ and an antiferromagnetic iron chalcogenide FeTe.

Spin–orbit coupling in noncentrosymmetric crystals leads to spin–momentum locking – a directional relationship between an electron’s spin angular momentum and its linear momentum. Isotropic orthogonal Rashba spin–momentum locking has been studied for decades, while its counterpart, isotropic parallel Weyl spin–momentum locking has remained elusive in experiments. Theory predicts ...

Alex Amato and Elvezio Morenzoni have published a new textbook entitled 'Introduction to Muon Spin Spectroscopy: Applications to Solid State and Material Sciences'. The book is ideal for a first course in muon spin spectroscopy (µSR), comes enriched with exercises and solutions to master the subject and includes practical examples to quantify key experimental parameters.

Charge density wave (CDW) orders in vanadium-based kagome metals have recently received tremendous attention, yet their origin remains a topic of debate. The discovery of ScV₆Sn₆, a bilayer kagome metal featuring an intriguing √3 × √3 × √3 CDW order, offers a novel platform to explore the underlying mechanism behind the unconventional CDW. Here we combine ...

The superconductivity in systems containing dispersionless (flat) bands is seemingly paradoxical, as traditional Bardeen-Cooper-Schrieffer theory requires an infinite enhancement of the carrier masses. However, the combination of flat and steep (dispersive) bands within the multiple band scenario might boost superconducting responses, potentially explaining high-temperature superconductivity in cuprates and metal hydrides. Here, we report ...

One of the recipes for realizing topological superconductivity calls for interfacing a topological insulator with a superconductor. In a variant of that approach, Yi et al. grew a heterostructure consisting of layers of a magnetic topological insulator, (Bi,Sb)₂Te₃ doped with chromium, and antiferromagnetic iron telluride. Neither of these materials is superconducting, but iron telluride is a parent compound for a family of iron-based superconductors. Interfacing the layers led to the appearance of superconductivity in the presence of ferromagnetism and topological band structure. This combination of properties makes the heterostructure a promising, although not yet proven, platform for observing chiral topological superconductivity.

Magnetostriction results from the coupling between magnetic and elastic degrees of freedom. Though it is associated with a relatively small energy, we show that it plays an important role in determining the site of an implanted muon, so that the energetically favorable site can switch on crossing a magnetic phase transition. This surprising effect is demonstrated in the cubic rocksalt antiferromagnet MnO which undergoes a magnetostriction-driven rhombohedral distortion at the Néel temperature T_N = 118 K. Above T_N ...

Understanding the degree to which charge-stripe, spin-stripe, and superconducting orders compete/coexist is paramount for elucidating the microscopic pairing mechanism in the cuprate high-temperature superconductors. We explore the tunability of magnetism, superconductivity, and crystal structure in the stripe phase of the cuprate La_2−xBa_xCuO₄, by employing complementary techniques under compressive uniaxial stress in the CuO₂ plane. Our results show a sixfold increase ...

We report on measurements of the in-plane magnetic penetration depth (λab) in single crystals of Sr₂RuO₄ down to ≃0.015  K by means of muon-spin rotation-relaxation. The linear temperature dependence of λ⁻²_ab for T≲0.7  K suggests the presence of nodes in the superconducting gap. This statement is further substantiated by observation of the Volovik effect, i.e., the reduction of λ⁻²_ab as a function of the applied magnetic field. The experimental zero-field ...

Charge ordered kagome lattices have been demonstrated to be intriguing platforms for studying the intertwining of topology, correlation, and magnetism. The recently discovered charge ordered kagome material ScV₆Sn₆ does not feature a magnetic groundstate or excitations, thus it is often regarded as a conventional paramagnet. Here, using advanced muon-spin rotation spectroscopy, we uncover an unexpected hidden magnetism of the charge order. We observe an enhancement ...

Kondo impurities provide a nontrivial probe to unravel the character of the excitations of a quantum spin liquid. In the S = 1/2 Kitaev model on the honeycomb lattice, Kondo impurities embedded in the spin-liquid host can be screened by itinerant Majorana fermions via gauge-flux binding. Here, we report experimental signatures of metallic-like Kondo screening at intermediate temperatures in the Kitaev honeycomb material α-RuCl₃ with dilute Cr³⁺ (S = 3/2) impurities.

The interplay between spin-orbit interaction and magnetic order is one of the most active research fields in condensed matter physics and drives the search for materials with novel, and tunable, magnetic and spin properties. Here we report on a variety of unique and unexpected observations in thin multiferroic Ge_1−xMn_xTe films.

Manipulating the spin state of thin layers of superconducting material is a promising route to generate dissipationless spin currents in spintronic devices. Approaches typically focus on using thin ferromagnetic elements to perturb the spin state of the superconducting condensate to create spin-triplet correlations. We have investigated simple structures that generate spin-triplet correlations without using ferromagnetic elements.

Kagome lattices are intriguing and rich platforms for studying the intertwining of topology, electron correlation, and magnetism. These materials have been subject to tremendous experimental and theoretical studies not only due to their exciting physical properties but also as systems that may solve critical technological problems. We will review recent experimental progress on superconductivity and magnetic fingerprints of charge order in several kagome-lattice systems from the local-magnetic probe point of view by utilizing muon-spin rotation under extreme conditions, i.e., hydrostatic pressure, ultra low temperature and high magnetic field.