Scientific Highlights: Research Division "Research with Neutrons and Muons"
Spin ice expands to higher orders
With experimental work demonstrating that the correlated ground state of the pyrochlore system Ce2Sn2O7 is a quantum liquid of magnetic octupoles, an international team led by PSI researcher Romain Sibille establishes a fundamentally new state of matter: higher-rank multipole ice.
A quantum liquid of magnetic octupoles on the pyrochlore lattice
With experimental work demonstrating that the correlated ground state of the pyrochlore system Ce2Sn2O7 is a quantum liquid of magnetic octupoles, an international team led by PSI researcher Romain Sibille establishes a fundamentally new state of matter: higher-rank multipole ice.
Reversible spin storage in metal oxide - fullerene heterojunctions
We show that hybrid MnOx/C60 heterojunctions can be used to design a storage device for spin-polarized charge: a spin capacitor. Hybridization at the carbon-metal oxide interface leads to spin-polarized charge trapping after an applied voltage or photocurrent. Strong electronic structure changes, including a 1-eV energy shift and spin polarization in the C60 lowest unoccupied molecular orbital, are then revealed by x-ray absorption spectroscopy, in agreement with density functional theory simulations.
Quantifying Diffusion through Interfaces of Lithium-Ion Battery Active Materials
Detailed understanding of charge diffusion processes in a lithium-ion battery is crucial to enable its systematic improvement. Experimental investigation of diffusion at the interface between active particles and the electrolyte is challenging but warrants investigation as it can introduce resistances that, for example, limit the charge and discharge rates. Here, we show an approach to study diffusion at interfaces using muon spin spectroscopy.
Current-driven magnetic domain-wall logic
Spin-based logic architectures provide nonvolatile data retention, near-zero leakage, and scalability, extending the technology roadmap beyond complementary metal–oxide–semiconductor logic. Architectures based on magnetic domain walls take advantage of the fast motion, high density, non-volatility and flexible design of domain walls to process and store information. Such schemes, however, rely on domain-wall manipulation and clocking using an external magnetic field, which limits their implementation in dense, large-scale chips.
Broken time-reversal symmetry in the topological superconductor UPt3
Topological properties of materials are of fundamental as well as practical importance. Of particular interest are unconven- tional superconductors that break time-reversal symmetry, for which the superconducting state is protected topologically and vortices can host Majorana fermions with potential use in quantum computing. However, in striking contrast to the unconventional A phase of superfluid 3He where chiral symmetry was directly observed, .....
Tracking down the mystery of matter
At the ultracold neutron source at PSI, researchers have measured a property of the neutron more precisely than ever before: its electric dipole moment. That's because the search is still on for an explanation of why, after the Big Bang, there was more matter than antimatter.
Short film of a magnetic nano-vortex
Using a newly developed imaging method, researchers were able to visualise the magnetic structure inside a material with nanoscale resolution. They succeeded in creating a short "film" consisting of seven movie frames that shows, for the first time in 3D, how tiny vortices of the magnetisation deep within a material change over time.
Observation of a Charge-Neutral Muon-Polaron Complex in Antiferromagnetic Cr2O3
We report a comprehensive muon spin rotation (μSR) study of the prototypical magnetoelectric antiferromagnet Cr2O3. We find the positively charged muon (μ+) occupies several distinct interstitial sites and displays a rich dynamic behavior involving local hopping, thermally activated site transitions, and the formation of a charge-neutral complex composed of a muon and an electron polaron.
A link between quantum magnetism and electronic band topology
Muon spin rotation experiments establish a quantitative link between the magnetic and topological electronic properties of the kagome magnet Co3Sn2S2 — and demonstrate effective ways for tuning these properties.
Tunable anomalous Hall conductivity through volume-wise magnetic competition in a topological kagome magnet
Magnetic topological phases of quantum matter are an emerging frontier in physics and material science. Along these lines, several kagome magnets have appeared as the most promising platforms. Here, we explore magnetic correlations in the kagome magnet Co3Sn2S2. Using muon spin-rotation, we present evidence for competing magnetic orders in the kagome lattice of this compound.
Possible room-temperature signatures of unconventional 4f-electron quantum criticality in YbMn6Ge6−xSnx
We investigate the Sn composition dependence of the Yb valence and local magnetization in YbMn6Ge6−xSnx (4.25 ≤x≤ 5.80) using x-ray absorption spectroscopy (XANES) and x-ray magnetic circular dichroism at the Yb L3 edge. In these materials, where Mn is ferromagnetically ordered, we observe a decrease of the Yb valence upon reducing the chemical pressure by Sn doping and a suppression of the Yb magnetic moment for strongly hybridized 4f states (ν ∼ 2.77).
Magnetism and anomalous transport in the Weyl semimetal PrAlGe: possible route to axial gauge fields
In magnetic Weyl semimetals, where magnetism breaks time-reversal symmetry, large magnetically sensitive anomalous transport responses are anticipated that could be useful for topological spintronics. The identification of new magnetic Weyl semimetals is therefore in high demand, particularly since in these systems Weyl node configurations may be easily modified using magnetic fields. Here we explore experimentally the magnetic semimetal PrAlGe, and unveil a direct correspondence between easy-axis Pr ferromagnetism and anomalous Hall and Nernst effects.
Well varnished violins play longer
Traditionally, violins are varnished to protect them from humidity and other environmental influences. At PSI, a scientific team has investigated how different coatings affect the instrument. Under no circumstances, they found, should anyone try to do without varnish completely.
Topological Magnetic Phase in the Candidate Weyl Semimetal CeAlGe
We report the discovery of topological magnetism in the candidate magnetic Weyl semimetal CeAlGe. Using neutron scattering we find this system to host several incommensurate, square-coordinated multi-k⃗ magnetic phases below TN. The topological properties of a phase stable at intermediate magnetic fields parallel to the c axis are suggested by observation of a topological Hall effect.
Modelling and simulation pay off
Researchers in PSI's Laboratory for Scientific Computing and Modelling solve the most complex problems through a combination of theory, modelling, and high-performance computing. With powerful computers, they simulate the smallest molecules or large research facilities.
Determination and evaluation of the nonadditivity in wetting of molecularly heterogeneous surfaces
Every folded protein presents an interface with water that is composed of domains of varying hydrophilicity/-phobicity. Many simulation studies have highlighted the nonadditivity in the wetting of such nanostructured surfaces in contrast with the accepted theoretical formula that is additive. We present here an experimental study on surfaces of identical composition but different organization of hydrophobic and hydrophilic domains.
Field-induced double spin spiral in a frustrated chiral magnet
Magnetic ground states with peculiar spin textures, such as magnetic skyrmions and multifunctional domains are of enormous interest for the fundamental physics governing their origin as well as potential applications in emerging technologies. Of particular interest are multiferroics, where sophisticated interactions between electric and magnetic phenomena can be used to tailor several functionalities.
The multi-layered physics of layered superconductors
Muon spin rotation experiments provide unique microscopic insight into the superconductivity and magnetism of transition metal dichalcogenides — and reveal complex and unconventional patterns, hinting towards a common mechanism for and electronic origin of ‘unconventional’ superconductivity.
Distortion mode anomalies in bulk PrNiO3: Illustrating the potential of symmetry-adapted distortion mode analysis for the study of phase transitions
The origin of the metal-to-insulator transition (MIT) in RNiO3 perovskites with R = trivalent 4f ion has challenged the condensed matter research community for almost three decades. A drawback for progress in this direction has been the lack of studies combining physical properties and accurate structural data covering the full nickelate phase diagram. Here we focus on a small region close to the itinerant limit (R = Pr, 1.5K < T < 300K), where we investigate the gap opening and the simultaneous emergence of charge order in PrNiO3.