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Laboratory for Waste Management (LES)

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2014

  • Aldaba D, Glaus M, Leupin O, Van Loon L, Vidal M, Rigol A
    Suitability of various materials for porous filters in diffusion experiments
    Radiochimica Acta. 2014; 102(8): 723-730. https://doi.org/10.1515/ract-2013-2176
    DORA PSI
  • Baeyens B, Marques Fernandes M, Bradbury MH
    Comparison between host rock and bentonite sorption measurements and predictions using the SDB approach applied in the provisional safety analyses for SGT-E2
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 12-05.
    DORA PSI
  • Baeyens B, Thoenen T, Bradbury MH, Marques Fernandes M
    Sorption data bases for argillaceous rocks and bentonite for the provisional safety analyses for SGT-E2
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 12-04.
    DORA PSI
  • Berner U
    Solubility of radionuclides in a bentonite environment for provisional safety analyses for SGT-E2
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 14-06.
    DORA PSI
  • Berner U
    Solubility of radionuclides in a concrete environment for provisional safety analyses for SGT-E2
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 14-07.
    DORA PSI
  • Bhatt JS, McDonald PJ, Faux DA, Howlett NC, Churakov SV
    NMR relaxation parameters from molecular simulations of hydrated inorganic nanopores
    International Journal of Quantum Chemistry. 2014; 114(18): 1220-1228. https://doi.org/10.1002/qua.24708
    DORA PSI
  • Bradbury MH, Berner U, Curti E, Hummel W, Kosakowski G, Thoenen T
    The long term evolution of the nearfield of the HLW repository
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 12-01.
    DORA PSI
  • Churakov SV, Labbez C, Pegado L, Sulpizi M
    Intrinsic acidity of surface sites in calcium silicate hydrates and its implication to their electrokinetic properties
    Journal of Physical Chemistry C. 2014; 118(22): 11752-11762. https://doi.org/10.1021/jp502514a
    DORA PSI
  • Churakov SV, Gimmi T, Unruh T, Van Loon LR, Juranyi F
    Resolving diffusion in clay minerals at different time scales: combination of experimental and modeling approaches
    Applied Clay Science. 2014; 96: 36-44. https://doi.org/10.1016/j.clay.2014.04.030
    DORA PSI
  • Curti E, Froideval-Zumbiehl A, Günther-Leopold I, Martin M, Bullemer A, Linder H, et al.
    Selenium redox speciation and coordination in high-burnup UO2 fuel: consequences for the release of 79Se in a deep underground repository
    Journal of Nuclear Materials. 2014; 453(1-3): 98-106. https://doi.org/10.1016/j.jnucmat.2014.07.003
    DORA PSI
  • Daehn R, Schaub P, Popov D, Maeder U, Wieland E
    Synchrotron-based micro X-ray diffraction investigations of cement-clay interfaces
    Presented at: International Mineralogical Association 2014; Johannesburg, South Africa.
    DORA PSI
  • Degueldre C, Pin S, Poonoosamy J, Kulik DA
    Redox state of plutonium in irradiated mixed oxide fuels
    Journal of Physics and Chemistry of Solids. 2014; 75(3): 358-365. https://doi.org/10.1016/j.jpcs.2013.11.001
    DORA PSI
  • Dilnesa BZ, Wieland E, Lothenbach B, Dähn R, Scrivener KL
    Fe-containing phases in hydrated cements
    Cement and Concrete Research. 2014; 58: 45-55. https://doi.org/10.1016/j.cemconres.2013.12.012
    DORA PSI
  • Dilnesa BZ, Lothenbach B, Renaudin G, Wichser A, Kulik D
    Synthesis and characterization of hydrogarnet Ca3(AlxFe1 - X)2(SiO4)y(OH)4(3 - y)
    Cement and Concrete Research. 2014; 59: 96-111. https://doi.org/10.1016/j.cemconres.2014.02.001
    DORA PSI
  • Dähn R, Popov D, Schaub P, Pattison P, Grolimund D, Mäder U, et al.
    X-ray micro-diffraction studies of heterogeneous interfaces between cementitious materials and geological formations
    Physics and Chemistry of the Earth. 2014; 70-71: 96-103. https://doi.org/10.1016/j.pce.2013.10.010
    DORA PSI
  • Gimmi T, Leupin OX, Eikenberg J, Glaus MA, Van Loon LR, Waber HN, et al.
    Anisotropic diffusion at the field scale in a 4-year multi-tracer diffusion and retention experiment - I: Insights from the experimental data
    Geochimica et Cosmochimica Acta. 2014; 125: 373-393. https://doi.org/10.1016/j.gca.2013.10.014
    DORA PSI
  • Hingerl FF, Wagner T, Kulik DA, Thomsen K, Driesner T
    A new aqueous activity model for geothermal brines in the system Na-K-Ca-Mg-H-Cl-SO4-H2O from 25 to 300°C
    Chemical Geology. 2014; 381: 78-93. https://doi.org/10.1016/j.chemgeo.2014.05.007
    DORA PSI
  • Hingerl FF, Kosakowski G, Wagner T, Kulik DA, Driesner T
    GEMSFIT: a generic fitting tool for geochemical activity models
    Computational Geosciences. 2014; 18(2): 227-242. https://doi.org/10.1007/s10596-014-9405-3
    DORA PSI
  • Jacques D, Lothenbach B, Wieland E
    Mechanisms and modelling of waste-cement and cement-host rock interactions
    Physics and Chemistry of the Earth. 2014; 70-71: 1-2. https://doi.org/10.1016/j.pce.2014.05.001
    DORA PSI
  • Kang J, Prasianakis NI, Mantzaras J
    Thermal multicomponent lattice Boltzmann model for catalytic reactive flows
    Physical Review E. 2014; 89(6): 063310 (13 pp.). https://doi.org/10.1103/PhysRevE.89.063310
    DORA PSI
  • Kosakowski G, Berner U, Wieland E, Glaus M, Degueldre C
    Geochemical evolution of the L/ILW near field
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 14-11.
    DORA PSI
  • Kosakowski G, Smith P
    Long-term evolution of the engineered gas transport system
    Wettingen: Nationale Genossenschaft für die Lagerung radioaktiver Abfälle (Nagra); 2014. Nagra Arbeitsberichte (NABs): 14-16.
    DORA PSI
  • Kosakowski G, Watanabe N
    OpenGeoSys-Gem: a numerical tool for calculating geochemical and porosity changes in saturated and partially saturated media
    Physics and Chemistry of the Earth. 2014; 70-71: 138-149. https://doi.org/10.1016/j.pce.2013.11.008
    DORA PSI
  • Kulasinski K, Keten S, Churakov SV, Derome D, Carmeliet J
    A comparative molecular dynamics study of crystalline, paracrystalline and amorphous states of cellulose
    Cellulose. 2014; 21(3): 1103-1116. https://doi.org/10.1007/s10570-014-0213-7
    DORA PSI
  • Kulasinski K, Keten S, Churakov SV, Guyer R, Carmeliet J, Derome D
    Molecular mechanism of moisture-induced transition in amorphous cellulose
    ACS Macro Letters. 2014; 3(10): 1037-1040. https://doi.org/10.1021/mz500528m
    DORA PSI
  • Lothenbach B, Rentsch D, Wieland E
    Hydration of a silica fume blended low-alkali shotcrete cement
    Physics and Chemistry of the Earth. 2014; 70-71: 3-16. https://doi.org/10.1016/j.pce.2013.09.007
    DORA PSI
  • Osán J, Kéri A, Breitner D, Fábián M, Dähn R, Simon R, et al.
    Microscale analysis of metal uptake by argillaceous rocks using positive matrix factorization of microscopic X-ray fluorescence elemental maps
    Spectrochimica Acta B: Atomic Spectroscopy. 2014; 91: 12-23. https://doi.org/10.1016/j.sab.2013.11.002
    DORA PSI
  • Pegado L, Labbez C, Churakov SV
    Mechanism of aluminium incorporation into C-S-H from ab initio calculations
    Journal of Materials Chemistry A. 2014; 2(10): 3477-3483. https://doi.org/10.1039/c3ta14597b
    DORA PSI
  • Pfingsten W
    The influence of stable element inventory on the migration of radionuclides in the vicinity of a high level nuclear waste repository exemplified for 59Ni
    Applied Geochemistry. 2014; 49: 103-115. https://doi.org/10.1016/j.apgeochem.2014.05.002
    DORA PSI
  • Puigmartí-Luis J, Rubio-Martínez M, Imaz I, Cvetković BZ, Abad L, Pérez del Pino A, et al.
    Localized, stepwise template growth of functional nanowires from an amino acid-supported framework in a microfluidic chip
    ACS Nano. 2014; 8(1): 818-826. https://doi.org/10.1021/nn4054864
    DORA PSI
  • Savoye S, Altmann S, Appelo T, Gaboreau S, Maes N, Schäfer T, et al.
    CATCLAY: "Processes of cation migration in clayrocks"
    In: Directorate-General for Research and Innovation, ed. Conference proceedings EURADWASTE '13. Vol. KI-NA-26-846-EN-N. EU publications. Luxembourg: Publications Office of the European Union; 2014:275-283.
    DORA PSI
  • Schumann D, Stowasser T, Volmert B, Günther-Leopold I, Linder H, Wieland E
    Determination of the 14C content in activated steel components from a neutron spallation source and a nuclear power plant
    Analytical Chemistry. 2014; 86(11): 5448-5454. https://doi.org/10.1021/ac500654a
    DORA PSI
  • Soler JM, Leupin OX, Gimmi T, Van Loon LR
    The DR-A in-situ diffusion experiment at Mont Terri: effects of changing salinity on diffusion and retention properties
    In: Duro L, Giménez J, Casas I, De Pablo J, eds. Symposium NW – scientific basis for nuclear waste management XXXVII. Vol. 1665. Materials research society symposium proceedings. Warrendale, Pennsylvania: Materials Research Society; 2014:63-69. https://doi.org/10.1557/opl.2014.629
    DORA PSI
  • Soltermann D, Marques Fernandes M, Baeyens B, Miehé-Brendlé J, Dähn R
    Competitive Fe(II)-Zn(II) uptake on a synthetic montmorillonite
    Environmental Science and Technology. 2014; 48(1): 190-198. https://doi.org/10.1021/es402783r
    DORA PSI
  • Soltermann D, Marques Fernandes M, Baeyens B, Dähn R, Joshi PA, Scheinost AC, et al.
    Fe(II) uptake on natural montmorillonites. I. Macroscopic and spectroscopic characterization
    Environmental Science and Technology. 2014; 48(15): 8688-8697. https://doi.org/10.1021/es501887q
    DORA PSI
  • Soltermann D, Baeyens B, Bradbury MH, Fernandes MM
    Fe(II) uptake on natural montmorillonites. II. Surface complexation modeling
    Environmental Science and Technology. 2014; 48(15): 8698-8705. https://doi.org/10.1021/es501902f
    DORA PSI
  • Thien BMJ
    A simple way to constrain the stoichiometry of secondary smectites upon aqueous glass alteration
    Applied Geochemistry. 2014; 42: 45-46. https://doi.org/10.1016/j.apgeochem.2014.01.002
    DORA PSI
  • Thien BMJ, Kulik DA, Curti E
    A unified approach to model uptake kinetics of trace elements in complex aqueous - solid solution systems
    Applied Geochemistry. 2014; 41: 135-150. https://doi.org/10.1016/j.apgeochem.2013.12.002
    DORA PSI
  • Thoenen T
    Speciation calculations supporting the sorption data bases for argillaceous rocks and bentonite for the provisional safety analyses for SGT-E2
    Wettingen: Nationale Genossenschaft für die Lagerung radioaktiver Abfälle (Nagra); 2014. Nagra Arbeitsberichte (NABs): 12-52.
    DORA PSI
  • Thoenen T, Hummel W, Berner U, Curti E
    The PSI/Nagra chemical thermodynamic database 12/07
    Wettingen: Nationale Genossenschaft für die Lagerung radioaktiver Abfälle (Nagra); 2014. Nagra Arbeitsberichte (NABs): 14-49.
    DORA PSI
  • Thoenen T, Hummel W, Berner U, Curti E
    The PSI/Nagra chemical thermodynamic database 12/07
    Villigen PSI, Switzerland: Paul Scherrer Institut; 2014. PSI Bericht: 14-04.
    DORA PSI
  • Tits J, Gaona X, Laube A, Wieland E
    Influence of the redox state on the neptunium sorption under alkaline conditions: batch sorption studies on titanium dioxide and calcium silicate hydrates
    Radiochimica Acta. 2014; 102(5): 385-400. https://doi.org/10.1515/ract-2013-2151
    DORA PSI
  • Tits J, Fujita T, Harfouche M, Dähn R, Tsukamoto M, Wieland E
    Radionuclide uptake by calcium silicate hydrates: case studies with Th(IV) and U(VI)
    Villigen: Paul Scherrer Institut; 2014. PSI Bericht: 14-03.
    DORA PSI
  • Torapava N, Ramebäck H, Curti E, Lagerkvist P, Ekberg C
    Recrystallization of 223Ra with barium sulfate
    Journal of Radioanalytical and Nuclear Chemistry. 2014; 301(2): 545-553. https://doi.org/10.1007/s10967-014-3170-6
    DORA PSI
  • Van Loon LR, Müller W
    A modified version of the combined in-diffusion/abrasive peeling technique for measuring diffusion of strongly sorbing radionuclides in argillaceous rocks: a test study on the diffusion of caesium in Opalinus Clay
    Applied Radiation and Isotopes. 2014; 90: 197-202. https://doi.org/10.1016/j.apradiso.2014.04.009
    DORA PSI
  • Van Loon LR
    Effective diffusion coefficients and porosity values for argillaceous rocks and bentonite: measured and estimated values for the provisional safety analysis fo SGT-E2
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 12-03.
    DORA PSI
  • Vespa M, Dähn R, Wieland E
    Competition behaviour of metal uptake in cementitious systems: an XRD and EXAFS investigation of Nd- and Zn-loaded 11 Å tobermorite
    Physics and Chemistry of the Earth. 2014; 70-71: 32-38. https://doi.org/10.1016/j.pce.2014.01.001
    DORA PSI
  • Wieland E, Lothenbach B, Glaus MA, Thoenen T, Schwyn B
    Influence of superplasticizers on the long-term properties of cement pastes and possible impact on radionuclide uptake in a cement-based repository for radioactive waste
    Applied Geochemistry. 2014; 49: 126-142. https://doi.org/10.1016/j.apgeochem.2014.04.002
    DORA PSI
  • Wieland E
    Sorption data base for the cementitious near field of L/ILW and ILW repositories for provisional safety analyses for SGT-E2
    Wettingen: National Cooperative for the Disposal of Radioactive Waste (Nagra); 2014. Nagra: technical report: 14-08.
    DORA PSI
  • Wu T, Wang H, Zheng Q, Zhao YL, Van Loon LR
    Diffusion behavior of Se(IV) and Re(VII) in GMZ bentonite
    Applied Clay Science. 2014; 101: 136-140. https://doi.org/10.1016/j.clay.2014.07.028
    DORA PSI

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Paul Scherrer Institut
Laboratory for Waste Management
Prof. Dr. Sergey Churakov
5232 Villigen PSI

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Deborah Schneider
Telephone: +41 56 310 24 17
E-mail: deborah.schneider@psi.ch

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Institute of Geological Sciences
Prof. Dr. Sergey Churakov
Baltzerstrasse 1+3
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