Scientific Highlights
Solid-state qubits: Forget about being clean, embrace mess
So says new recipe for dense arrays of qubits with long lifetimes.
Observing laser-induced recrystallization
Synchrotron X-ray diffraction sheds light on laser-induced local recrystallization .
Field-induced bound-state condensation and spin-nematic phase in SrCu2(BO3)2 revealed by neutron scattering up to 25.9 T
In quantum magnetic materials, ordered phases induced by an applied mag- netic field can be described as the Bose-Einstein condensation (BEC) of mag- non excitations. In the strongly frustrated system SrCu2(BO3)2, no clear magnon BEC could be observed, pointing to an alternative mechanism, but the high fields required to probe this physics have remained a barrier to detailed investigation.Here we exploit the first purpose-built high-field neutron scattering facility to measure ...
Water-assisted generation of catalytic interface: The case of interfacial Pt-FeOx(OH)y sites active in preferential carbon monoxide oxidation
Pt-FeOx(OH)y interface with enhanced activity for PROX is generated via strong metal-support interaction. Increase in the degree of hydroxylation of Pt-FeOx(OH)y interface enhances the rate of PROX mediated by active Fe2+ species.
Designing the stripe-ordered cuprate phase diagram through uniaxial-stress
Understanding the degree to which charge-stripe, spin-stripe, and superconducting orders compete/coexist is paramount for elucidating the microscopic pairing mechanism in the cuprate high-temperature superconductors. We explore the tunability of magnetism, superconductivity, and crystal structure in the stripe phase of the cuprate La2−xBaxCuO4, by employing complementary techniques under compressive uniaxial stress in the CuO2 plane. Our results show a sixfold increase ...
Climate-neutral aviation: will it fly?
The European aviation sector stands at a pivotal juncture in its quest to achieve net-zero climate impacts. Focusing on flight CO2 emissions overlooks up to 80% of the sector's climate repercussions.
Our research delves deep into the role of electricity-based synthetic jet fuels and direct air carbon capture and storage (DACCS) as potential game-changers. These solutions promise climate-neutral aviation, but there's a catch: the relentless rise in air traffic. Relying solely on renewables-derived synthetic fuels may strain both economic and natural resources. On the flip side, offsetting fossil jet fuel impacts via DACCS poses its own set of challenges. Our findings underscore one clear message: for a genuinely climate-neutral European aviation, we must reconsider the scale of air traffic.
Quantification of PEFC Catalyst Layer Saturation via Small-Angle X‑ray Scattering
The complex nature of liquid water saturation in polymer electrolyte fuel cell (PEFC) catalyst layers (CLs) greatly affects the device performance. To investigate this problem, a method to quantify the presence of liquid water in a PEFC CL using small-angle X-ray scattering (SAXS) was developed in a collaboration of researchers of the Federal Institute for Materials Research and Testing (BAM, Berlin, Germany), the Photon Science Division and the Electrochemistry Laboratory of PSI. The method leverages the differences in electron densities between the solid catalyst matrix and the CL-pores filled with liquid water under dry and wet conditions, respectively.
Dichotomous Electrons: Travelling without Moving
Neutron scattering experiments give new understanding of how localized and free-flowing electrons collaborate to create material functionality.
Tetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular AFM Co1/3TaS2
The triangular lattice antiferromagnet (TLAF) has been the standard paradigm of frustrated magnetism for several decades. The most common magnetic ordering in insulating TLAFs is the 120° structure. However, a new triple-Q chiral ordering can emerge in metallic TLAFs, representing the short wave- length limit of magnetic skyrmion crystals. We report the metallic TLAF Co1/3TaS2 as the first example of tetrahedral triple-Q magnetic ordering with the associated topological Hall effect (non-zero σxy(H = 0)). We also ...
Phonon Topology and Winding of Spectral Weight in Graphite
The topology of electronic and phonon band structures of graphene is well studied and known to exhibit a Dirac cone at the K point of the Brillouin zone. Here, we applied inelastic x-ray scattering (IXS) along with ab initio calculations to investigate phonon topology in graphite, the 3D analog of graphene. We identified a pair of modes that form a very weakly gapped linear anticrossing at the K point that can be essentially viewed as a Dirac cone approximant. The IXS intensity ...