Laboratory for Non-linear Optics (LNO)

Scientists pioneer an approach called self-referenced streaking, clocking Auger electrons with sub-femtosecond resolution. The breakthrough will unlock the broader potential for attosecond time resolution at X-ray free-electron lasers

Excitation of coherent phonons using light is an emerging approach for investigating condensed matter physics. It has the potential not only to reveal the dynamics of collective lattice vibrations but also to tailor them for the ultrafast control over the electronic, magnetic, and structural properties in solids. The optical phonons, in most solids, lie primarily in the spectral region between 1 and 10 THz. Unlike conventional laser sources, coherent radiation at these frequencies allows us to study time-resolved lattice displacements with only minor deposition of heat or generation of hot electrons. However, the available high-field terahertz sources, with their quasi-single cycle temporal shape and broadband spectrum, cannot be used to excite the individual phonon modes. By contrast, the challenge of understanding the transient dynamics of low-energy excitations calls for novel sources of narrow-band terahertz radiation at high intensities that can be tuned to the individual phonon resonances. Moreover, with strong enough fields tuned precisely to a phonon resonance, non-linearities in the material can be targeted and potentially exploited.