Nanoscale sub-100 picosecond all-optical magnetization switching in GdFeCo microstructure

Magnetization dynamics inside a 5 µm x 5 µm structure.
(a) Time-resolved PEEM images using XMCD as a magnetic contrast mechanism recorded at a given time delay t after the laser pulse and
(b) extracted XMCD contrast as a function of the time delay t for three different ROI, defined in the inset image by the coloured area superimposed on the non-dichroic X-ray absorption of the structure. The 0° incoming laser direction with respect to the structure edge is indicated in the inset by the laser in-plane wave vector k. The corresponding inward (x) or outward (⋅) out-of-plane magnetization component M are indicated on the XMCD axis. The incoming laser fluence was F=5.1mJcm−2.

Ultrafast magnetization reversal driven by femtosecond laser pulses has been shown to be a promising way to write information. Seeking to improve the recording density has raised intriguing fundamental questions about the feasibility of combining ultrafast temporal resolution with sub-wavelength spatial resolution for magnetic recording. Here we report on the experimental demonstration of nanoscale sub-100 ps all-optical magnetization switching, providing a path to sub-wavelength magnetic recording. Using computational methods, we reveal the feasibility of nanoscale magnetic switching even for an unfocused laser pulse. This effect is achieved by structuring the sample such that the laser pulse, via both refraction and interference, focuses onto a localized region of the structure, the position of which can be controlled by the structural design. Time-resolved photo-emission electron microscopy studies reveal that nanoscale magnetic switching employing such focusing can be pushed to the sub-100 ps regime.